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Fonds consists of correspondence, financial records, diaries, travel diaries, calendars, sketch books, sketches and drawings, programmes and invitations pertaining to shows and exhibitions, inventories, speeches, awards, miscellaneous and printed material, photographs, slides and sound recordings covering all aspects of his life as a student, teacher, traveller, world-renowned artist and chronicler of the country he loved. There is also a small amount of material created and maintained by Ruth Collier (nee Brown) and some family genealogy files.

The fonds consists of correspondence, scrapbooks, news clippings, transcripts of local diaries, and alphabetical family and genealogical files. These genealogical files, which relate mainly to Bay of Quinte and Loyalist families, contain correspondence, research from printed sources, newspaper clippings and some photographs. Also included is a set of ordnance survey maps of Kingston and area dated 1869.

The fonds consists of correspondence, diaries and photographs from the period of Dunsmore's World War I service (1915-1919), and the WWI diaries of his brother-in-law Clarence Voaden (1917-1918). It also includes various writings, correspondence, lectures and addresses from his time of service on the Board of Trustees, and minutes and reports from the Queen's University Campus Planning committee as he also served on that committee for almost twenty years.