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The fonds consists of correspondence, memoranda, diaries, material by and about J.W. Dafoe, subject files, scrapbooks and miscellaneous pamphlets. The correspondence files, arranged chronologically, contain memoranda of confidential interviews on Canadian politics, trade, the economy, external affairs, defence. Often these memoranda are in the form of letters or vice versa, so the two have been filed together. The Diaries written by Grant Dexter in 1938-39 while he was in England touch on many aspects of Canadian External Affairs. Also included is a diary kept by Grant Dexter's wife Alice, outlining their life in London in 1937.

The fonds consists of correspondence, subject files, writings, addresses, and speeches relating to connections with major Canadian companies, Canadian Wartime Prices and Trade Board, 1940-5, and Royal Commission on Banking and Finances, 1961-63. There is also a collection of diaries that cover the period 1966 to 1982, however, they are, for the most part, daily calendars showing appointments and meetings. In addition, there is a list of the Queen's University Board of Trustees names, including Chairman J.D. Gibson. As well as a ballot for the election of a new member of the Board of Trustees.

The Margaret Phipps-Walker sous-fonds details a good deal of Mrs. Phipps-Walker's public career in Kingston and is especially strong in material about the Association of Women Electors. There is also a good deal of personal material, such as letters. While one had to 'read between the lines' to find much of Edward's feelings; Margaret's records show a more introspective side to her nature and include diaries written in the later years of her life.